The Sharpness enchantment increases the amount of attack damage dealt to a player or mob. You can add the Sharpness enchantment to any sword or axe using an enchanting table, anvil, or game command. Sharpness is effective against all mobs, not just undead ones. Sharpness would be the best enchantment to use out of the two since Smite would be useless when fighting other players or other mobs besides the undead. Since players can only choose one, Sharpness is the best choice.
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